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Reactive Al-O-Al sites in a natural zeolite: Triple-quantum oxygen-17 nuclear magnetic resonance
Reactive Al-O-Al sites natural zeolite Triple-quantum oxygen-17 nuclear magnetic resonance
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2012/4/1
In framework aluminosilicate materials (e.g., feldspars, zeolites and many others), it is generallyassumed that AlOtetrahedra do not share corners, i.e., that Al-O-Al oxygen sites are avoided whenstoi...
Three- and five-quantum 17O MAS NMR of forsterite Mg2SiO4
Three- and five-quantum 17O MAS NMR forsterite Mg2SiO4
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2012/3/31
17Three- and five-quantum O MAS NMR experiments are used to resolve fully the three crystallo-
graphically distinct oxygen species in forsterite (Mg
SiO ). The chemical shift and quadrupolar pa-2 4...
Disorder among network-modifier cations in silicate glasses: New constraints from triple-quantum 17O NMR
Disorder network-modifier cations silicate glasses New constraints triple-quantum 17O NMR
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2012/4/6
Thestateoforderingamongnetwork-modi?ercationsinmoltensilicateshasapoten-tiallylargeeffectontheiroverallcon?gurationalentropy,onfreeenergiesofmixing,and
onviscosityanddiffusivity.Mostmodelsofthermodyn...
Mechanism of CO32- substitution in carbonate-fluorapatite: Evidence from FTIR spectroscopy, 13C NMR, and quantum mechanical calculations---Reply to Nathan
Mechanism CO32- substitution carbonate-fluorapatite Evidence FTIR spectroscopy 13C NMR quantum mechanical calculations---Reply Nathan
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2012/4/5
In the critical comment byNathan (1996), the author essentially claims that the samples used in our study (Regnier et al. 1994) werenot very appropriate to dem-onstrate the absence of C03P-. Furthermo...
Mechanism of CO32- substitution in carbonate-fluorapatite: Evidence from FTIR spectroscopy, 13C NMR, and quantum mechanical calculations---Discussion
Mechanism CO32- substitution carbonate-fluorapatite Evidence FTIR spectroscopy 13C NMR quantum mechanical calculations---Discussion
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2012/4/5
The carbonate substitution in apatite continues to pro-voke controversies. In a recent paper, Regnier etal. (1994) challenged the existence of the hypothetical C03P- ion in carbonate-fluorapatite (fra...